1. Nanoelectronics

  • Non-invasive atomic layer etching. A protocol is devised that allows for non-invasive and atomically digital etching of van der Waals transition-metal dichalcogenides through selective alloying via low-temperature thermal diffusion and subsequent wet etching, representing a highly precise and non-invasive tailoring route for material manipulation. See Nat. Commun. 13, 1844 (2022).
  • An air-gapped FET. By using van der Waals stacking method, we fabricated semi-suspended, ari-gapped FETs with negligible scanning hystersis and high carrier mobilities. See Appl. Phys. Lett. 121, 023503 (2022).
  • Clean BN-Encapsulated 2D FETs. We managed to integrate lithography-defined contacts into BN-encapsulated 2D FETs, giving rise to high overall device quality comparable to the state-of-the-art results. See ACS AMI 14, 18697 (2022).
  • On-chip integration of patterned 2D materials. We developed an novel subsidence-assisted integration method that enables spatially precise integration of arrays of micropatterned 2D crystals onto Si/SiO2 substrates, representing an attractive, low-cost system-on-chip strategy toward More-than-Moore microelectronics. See ACS Nano. 13, 2654 (2019).
  • Graphene voltage inverters. We exploited the spontaneous surface passivation of Al to define the gate/dielectric stacks and fabricated complementary-like voltage inverters based on ambipolar graphene transistors, with over-unity voltage gains and matched input and output. See Nano Lett. 10, 2357 (2010); ACS Nano. 5, 500 (2011); Small 7, 1552 (2011).

2. Device physics in FETs

  • Theory of charge scattering. We developed a generalized Coulomb scattering model with strictly considering device configurative conditions, that is, asymmetric dielectric environments and lopsided carrier distribution in 2D FETs, to accurately describe the carrier scattering process [J. Phys. Soc. Jpn., 84, 121011 (2015)] and the origin of the thinning-induced mobility degradation [ Nano Lett., 22, 6671(2022), Nano Lett. 13, 3546 (2013)]. This understanding highlights the critical role of surface quality in electrical transport. A review on charge transport in 2D FETs can be found at Chem. Soc. Rev., 45, 118 (2016).
  • Metal/Semiconductor contact. We investigated the thickness scaling effect on the charge injection barrier at Au/MoS2 interfaces and observed the thickness reduction induced crossover of electrical contact therein. [ACS Nano, 8, 12836 (2014)]. In WS2 FETs with low-work-function metal ytterbium (Yb) as contacts, we clarified the presence of significant tunneling injection that invalidates the thermionic emission model for barrier estimation. [Appl. Phys. Lett., 120, 253505 (2022)].
  • Thickness identification of 2D crystals. We observed strong optical inteference and its effect on Raman intensity in the layered structures, which can be used to predict quantitative Raman spectra and to count thickness of atomic layers on insulating substrates. See ACS Nano, 6, 7381 (2012).